Nonlinear Fano interferences in open quantum systems: An exactly solvable model

Daniel Finkelstein-Shapiro, Monica Calatayud, Osman Atabek, Vladimiro Mujica, and Arne Keller
Phys. Rev. A 93, 063414 – Published 16 June 2016
PDFHTMLExport Citation

Abstract

We obtain an explicit solution for the stationary-state populations of a dissipative Fano model, where a discrete excited state is coupled to a continuum set of states; both excited sets of states are reachable by photoexcitation from the ground state. The dissipative dynamic is described by a Liouville equation in Lindblad form and the field intensity can take arbitrary values within the model. We show that the population of the continuum states as a function of laser frequency can always be expressed as a Fano profile plus a Lorentzian function with effective parameters whose explicit expressions are given in the case of a closed system coupled to a bath as well as for the original Fano scattering framework. Although the solution is intricate, it can be elegantly expressed as a linear transformation of the kernel of a 4×4 matrix which has the meaning of an effective Liouvillian. We unveil key notable processes related to the optical nonlinearity and which had not been reported to date: electromagnetic-induced transparency, population inversions, power narrowing and broadening, as well as an effective reduction of the Fano asymmetry parameter.

  • Figure
  • Figure
  • Figure
  • Figure
  • Received 15 September 2015
  • Revised 24 February 2016

DOI:https://doi.org/10.1103/PhysRevA.93.063414

©2016 American Physical Society

Physics Subject Headings (PhySH)

Atomic, Molecular & OpticalGeneral Physics

Authors & Affiliations

Daniel Finkelstein-Shapiro1,2,3,*, Monica Calatayud2,3,4, Osman Atabek5, Vladimiro Mujica1, and Arne Keller5

  • 1Department of Chemistry and Biochemistry, Arizona State University, Tempe Arizona 85282, USA
  • 2Sorbonne Universités, UPMC Univ Paris 06, UMR 7616, Laboratoire de Chimie Théorique, F-75005, Paris, France
  • 3CNRS, UMR 7616, Laboratoire de Chimie Théorique, F-75005, Paris, France
  • 4Institut Universitaire de France, France
  • 5Institut des Sciences Moléculaires d'Orsay, Bâtiment 350, UMR8214, CNRS-Univ. Paris-Sud, Univ. Paris-Saclay 91405 Orsay, France

  • *dfinkel2@asu.edu

Article Text (Subscription Required)

Click to Expand

Supplemental Material (Subscription Required)

Click to Expand

References (Subscription Required)

Click to Expand
Issue

Vol. 93, Iss. 6 — June 2016

Reuse & Permissions
Access Options
CHORUS

Article Available via CHORUS

Download Accepted Manuscript
Author publication services for translation and copyediting assistance advertisement

Authorization Required


×
×

Images

×

Sign up to receive regular email alerts from Physical Review A

Log In

Cancel
×

Search


Article Lookup

Paste a citation or DOI

Enter a citation
×